Sediments as sinks and sources of marine radionuclides: Implications for their use as ocean tracers.

A Lagrangian transport model for the North Atlantic has been applied to simulate the historical releases of 137Cs, 129I and 236U from the European nuclear fuel reprocessing plants. Advection by currents, mixing and decay are included, as radionuclide interactions between water, sediments and suspended matter. The model was validated comparing predictions with measured radionuclide concentrations in water and sediments in several areas. 129I and 236U signals entering the Arctic Ocean have been compared with the input terms: the 236U signal is distorted, but the 129I signal preserves its shape. In the first moments after the releases, the sediments act as sinks for 236U, but not significantly for 129I and ultimately they become sources of 236U to the open sea. This results in a weaker correlation between input and output signals for 236U than for 129I. The same effects as for 236U have been found for 137Cs signal into the Arctic.

Tracing the upwelling process in the northern Benguela upwelling system (nBUS) by 129I.

New data on the presence of 129I in seawater in the Southern Hemisphere measured by Accelerator Mass Spectrometry (AMS) is presented. The samples were collected in 2014 along the Namibian coast during a cruise organised by the National Marine Information and Research Centre (NatMIRC), the national laboratories of the Ministry of Fisheries and Marine Resources (MFMR) in Namibia, and the IAEA Environment Laboratories (IAEA NAEL) in Monaco. The Benguela upwelling system is known as one of the most important marine upwelling regions in the world. Strong winds induce an offshore transport of surface seawater which is substituted by cool subsurface water inshore. As this water is nutrient-rich, which leads to high primary productivity, the Benguela upwelling system has a very important role as a fishing production area. The 129I concentrations in samples were between (0.66 ± 0.14) × 107 and (1.45 ± 0.30) × 107 atoms/kg. The highest 129I concentrations were found in the offshore surface samples. Deep-sea and inshore samples contained lower 129I concentrations, possibly as an effect of the upwelling process. A comparison with previously published studies suggests that the presence of 129I in the northern Benguela upwelling system (nBUS), is mainly due to the impact of nuclear weapons global fallout, without any evident impact of nuclear fuel reprocessing.

Recent evolution of 129I levels in the Nordic Seas and the North Atlantic Ocean.

Most of the anthropogenic radionuclide 129I released to the marine environment from the nuclear fuel reprocessing plants (NFRP) at Sellafield (England) and La Hague (France) is transported to the Arctic Ocean via the North Atlantic Current and the Norwegian Coastal Current. 129I concentrations in seawater provides a powerful and well-established radiotracer technique to provide information about the mechanisms which govern water mass transport in the Nordic Seas and the Arctic Ocean and is gaining importance when coupled with other tracers (e.g. CFC, 236U). In this work, 129I concentrations in surface and depth profiles from the Nordic Seas and the North Atlantic (NA) Ocean collected from four different cruises between 2011 and 2012 are presented. This work allowed us to i) update information on 129I concentrations in these areas, required for the accurate use of 129I as a tracer of water masses; and ii) investigate the formation of deep water currents in the eastern part of the Nordic Seas, by the analysis of 129I concentrations and temperature-salinity (T-S) diagrams from locations within the Greenland Sea Gyre. In the Nordic Seas, 129I concentrations in seawater are of the order of 109 at·kg-1, one or two orders of magnitude higher than those measured at the NA Ocean, not so importantly affected by the releases from the NFRP. 129I concentrations of the order of 108atoms·kg-1 at the Ellet Line and the PAP suggest a direct contribution from the NFRP in the NA Ocean. An increase in the concentrations in the Nordic Seas between 2002 and 2012 has been detected, which agrees with the temporal evolution of the 129I liquid discharges from the NFRPs in years prior to this. Finally, 129I profile concentrations, 129I inventories and T-S diagrams suggest that deep water formation occurred in the easternmost area of the Nordic Seas during 2012.